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Chemical Dynamics in Condensed Phases
Relaxation, Transfer and Reactions in Condensed Molecular Systems
Abraham Nitzan
744 pages
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95 line drawings
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240x168mm
978-0-19-852979-8
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Hardback
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06 April 2006
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- First book providing introduction to metals, semiconductors, and their interfaces with molecular systems
- Covers, under one consistent framework, traditional subjects like electron transfer and electrode kinetics and very new subjects such as molecular conduction
- Comprehensive coverage of the effect of thermal environment on relaxation, charge and energy transfer, reaction dynamics, and spectroscopy in molecular systems
- Introductory material (1) Quantum dynamics in the Schrödinger and Liouville formalisms and (2) Stochastic theory of physical and chemical (and biological) processes, has not been given at this level before
- Class-tested, based on teaching of various courses
This text provides a uniform and consistent approach to diversified problems encountered in the study of dynamical processes in condensed phase molecular systems. Given the broad interdisciplinary aspect of this subject, the book focuses on three themes: coverage of needed background material, in-depth introduction of methodologies, and analysis of several key applications. The uniform approach and common language used in all discussions help to develop general understanding and insight on condensed phases chemical dynamics. The applications discussed are among the most fundamental processes that underlie physical, chemical and biological phenomena in complex
systems.
The first part of the book starts with a general review of basic mathematical and physical methods (Chapter 1) and a few introductory chapters on quantum dynamics (Chapter 2), interaction of radiation and matter (Chapter 3) and basic properties of solids (chapter 4) and liquids (Chapter 5). In the second part the text embarks on a broad coverage of the main methodological approaches. The central role of classical and quantum time correlation functions is emphasized in Chapter 6. The presentation of dynamical phenomena in complex systems as stochastic processes is discussed in Chapters 7 and 8. The basic theory of quantum relaxation phenomena is developed in Chapter 9, and carried on in Chapter 10 which introduces the density operator, its quantum evolution
in Liouville space, and the concept of reduced equation of motions. The methodological part concludes with a discussion of linear response theory in Chapter 11, and of the spin-boson model in chapter 12. The third part of the book applies the methodologies introduced earlier to several fundamental processes that underlie much of the dynamical behaviour of condensed phase molecular systems. Vibrational relaxation and vibrational energy transfer (Chapter 13), Barrier crossing and diffusion controlled reactions (Chapter 14), solvation dynamics (Chapter 15), electron transfer in bulk solvents (Chapter 16) and at electrodes/electrolyte and metal/molecule/metal junctions (Chapter 17), and several processes pertaining to molecular spectroscopy in condensed phases (Chapter 18) are the main
subjects discussed in this part.Readership: Advanced undergraduate and graduate students in physics and chemistry. Faculty and students who are engaged in research and development involving chemical reaction dynamics, relaxation and transport phenomena in condensed phases and interfaces.
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Abraham Nitzan, Department of Chemistry, Tel Aviv University
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"'Beautifully and clearly written, describing mathematics in necessary detail without overloading the reader, and very neatly and consisely explaining physics of the described phenomena.' European Journal of Chemical Physics and Physical Chemistry, August 2007" "This is an excellent book which is intended to be a text for a graduate course in condensed matter chemistry and physics. It is extremely well written from the pedagogic and literary points of view. I particularly enjoyed the extremely pertinent quotations from Lucretius at the begining of each chapter. Journal of Statistical Physics, Vol. 126, No. 6, March 2007, Irwin Oppenheim, Massachusett Institute of Technology, USA"
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Part I: Background
1: Review of some mathematical and physical subjects
2: Quantum Dynamics using the time dependent Schrödinger equation
3: An overview of quantum electrodynamics and matter radiation-field interaction
4: Introduction to solids
5: Introduction to liquids
Part II: Methods
6: Time correlation functions
7: Introduction to Stochastic processes
8: Stochastic equations of motion
9: Introduction to quantum relaxation processes
10: The quantum mechanical density operator and its time evolution: Quantum dynamics from the quantum Liouville equation
11: Linear response theory
12: The spin-boson model
Part III: Applications
13: Vibrational energy relaxation
14: Chemical reactions in Condensed Phases
15: Solvation dynamics
16: Electron transfer processes
17: Electron transfer and transmission at molecule-metal and molecule-semiconductor interfaces
18: Spectroscopy
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The specification in this catalogue, including without limitation price, format, extent, number of illustrations, and month of publication, was as accurate as possible at the time the catalogue was compiled. Occasionally, due to the nature of some contractual restrictions, we are unable to ship a specific product to a particular territory. Jacket images are provisional and liable to change before publication.
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